{"database":"biostudies-literature","file_versions":[],"scores":null,"additional":{"omics_type":["Unknown"],"volume":["17(1)"],"submitter":["Wang C"],"pubmed_abstract":["Artificial carbon fixation is a promising pathway for achieving the carbon cycle and environment remediation. However, the sluggish kinetics of oxygen evolution reaction (OER) and poor selectivity of CO<sub>2</sub> reduction seriously limited the overall conversion efficiencies of solar energy to chemical fuels. Herein, we demonstrated a facile and feasible strategy to rationally regulate the coordination environment and electronic structure of surface-active sites on both photoanode and cathode. More specifically, the defect engineering has been employed to reduce the coordination number of ultrathin FeNi catalysts decorated on BiVO<sub>4</sub> photoanodes, resulting in one of the highest OER activities of 6.51 mA cm<sup>-2</sup> (1.23 V<sub>RHE</sub>, AM 1.5G). Additionally, single-atom "],"journal":["Nano-micro letters"],"pagination":["184"],"full_dataset_link":["https://www.ebi.ac.uk/biostudies/studies/S-EPMC11904044"],"repository":["biostudies-literature"],"pubmed_title":["Highly Active Oxygen Evolution Integrating with Highly Selective CO&lt;sub&gt;2&lt;/sub&gt;-to-CO Reduction."],"pmcid":["PMC11904044"],"pubmed_authors":["Wang C","Geng L","Bi Y"],"additional_accession":[]},"is_claimable":false,"name":"Highly Active Oxygen Evolution Integrating with Highly Selective CO&lt;sub&gt;2&lt;/sub&gt;-to-CO Reduction.","description":"Artificial carbon fixation is a promising pathway for achieving the carbon cycle and environment remediation. However, the sluggish kinetics of oxygen evolution reaction (OER) and poor selectivity of CO<sub>2</sub> reduction seriously limited the overall conversion efficiencies of solar energy to chemical fuels. Herein, we demonstrated a facile and feasible strategy to rationally regulate the coordination environment and electronic structure of surface-active sites on both photoanode and cathode. More specifically, the defect engineering has been employed to reduce the coordination number of ultrathin FeNi catalysts decorated on BiVO<sub>4</sub> photoanodes, resulting in one of the highest OER activities of 6.51 mA cm<sup>-2</sup> (1.23 V<sub>RHE</sub>, AM 1.5G). Additionally, single-atom ","dates":{"release":"2025-01-01T00:00:00Z","publication":"2025 Mar","modification":"2026-03-27T16:46:00.726Z","creation":"2025-04-03T23:26:33.226Z"},"accession":"S-EPMC11904044","cross_references":{"pubmed":["40074988"],"doi":["10.1007/s40820-025-01688-2"]}}