{"database":"biostudies-literature","file_versions":[],"scores":null,"additional":{"submitter":["Fu S"],"funding":["Natural Science Foundation of Shandong Province (Shandong Provincial Natural Science Foundation)","National Natural Science Foundation of China (National Science Foundation of China)","Taishan Scholar Foundation of Shandong Province"],"pagination":["1457-1464"],"full_dataset_link":["https://www.ebi.ac.uk/biostudies/studies/S-EPMC12404993"],"repository":["biostudies-literature"],"omics_type":["Unknown"],"volume":["24(9)"],"pubmed_abstract":["Hot carriers, inheriting excess kinetic energy from high-energy photons, drive numerous optoelectronic applications reliant on non-equilibrium transport processes. Although extensively studied in inorganic materials, their potential in organic-based systems remains largely unexplored. Here we demonstrate highly mobile hot carriers in crystalline two-dimensional conjugated coordination polymer Cu<sub>3</sub>BHT (BHT, benzenehexathiol) films. Leveraging a suite of ultrafast spectroscopic and imaging techniques, we map the microscopic charge transport landscape in Cu<sub>3</sub>BHT films following non-equilibrium photoexcitation across temporal, spatial and frequency domains, revealing two distinct high-mobility transport regimes. In the non-equilibrium regime, hot carriers achieve an ultrahi"],"journal":["Nature materials"],"pubmed_title":["Unveiling high-mobility hot carriers in a two-dimensional conjugated coordination polymer."],"pmcid":["PMC12404993"],"funding_grant_id":["tsqn201909047","22472085","ZR2023JQ005","22272092"],"pubmed_authors":["Hambsch M","Fu S","Zhang J","Liu M","Feng X","Zhang H","Kaiser U","Gao G","Li K","Dong R","Zhang W","Parkin SSP","Bonn M","Huang X","Gao L","St Petkov P","Gao W","Mannsfeld SCB","Wang Z","Zhu T","Wang HI"],"additional_accession":[]},"is_claimable":false,"name":"Unveiling high-mobility hot carriers in a two-dimensional conjugated coordination polymer.","description":"Hot carriers, inheriting excess kinetic energy from high-energy photons, drive numerous optoelectronic applications reliant on non-equilibrium transport processes. Although extensively studied in inorganic materials, their potential in organic-based systems remains largely unexplored. Here we demonstrate highly mobile hot carriers in crystalline two-dimensional conjugated coordination polymer Cu<sub>3</sub>BHT (BHT, benzenehexathiol) films. Leveraging a suite of ultrafast spectroscopic and imaging techniques, we map the microscopic charge transport landscape in Cu<sub>3</sub>BHT films following non-equilibrium photoexcitation across temporal, spatial and frequency domains, revealing two distinct high-mobility transport regimes. In the non-equilibrium regime, hot carriers achieve an ultrahi","dates":{"release":"2025-01-01T00:00:00Z","publication":"2025 Sep","modification":"2026-05-29T21:45:24.359Z","creation":"2026-04-08T06:08:40.43Z"},"accession":"S-EPMC12404993","cross_references":{"pubmed":["40360871"],"doi":["10.1038/s41563-025-02246-2"]}}