{"database":"biostudies-literature","file_versions":[],"scores":null,"additional":{"omics_type":["Unknown"],"volume":["9(36)"],"submitter":["Bahuguna G"],"pubmed_abstract":["Efficient neutral water splitting may represent in future a sustainable solution to unconstrained energy requirements, but yet necessitates the development of innovative avenues for achieving the currently unmet required performances. Herein, a novel paradigm based on the combination of electronic structure engineering and surface morphology tuning of earth-abundant 3D-hierarchical binder-free electrocatalysts is demonstrated, via a scalable single-step thermal transformation of nickel substrates under sulfur environment. A temporal-evolution of the resulting 3D-nanostructured substrates is performed for the intentional enhancement of non-abundant highly-catalytic Ni<sup>3+</sup> and pS<sub>n</sub> <sup>2-</sup> species on the catalyst surface, concomitantly accompanied with densification "],"journal":["Advanced science (Weinheim, Baden-Wurttemberg, Germany)"],"pagination":["e2203678"],"full_dataset_link":["https://www.ebi.ac.uk/biostudies/studies/S-EPMC9798964"],"repository":["biostudies-literature"],"pubmed_title":["Electronic Structure Engineering of Highly-Scalable Earth-Abundant Multi-Synergized Electrocatalyst for Exceptional Overall Water Splitting in Neutral Medium."],"pmcid":["PMC9798964"],"pubmed_authors":["Cohen A","Bahuguna G","Filanovsky B","Patolsky F"],"additional_accession":[]},"is_claimable":false,"name":"Electronic Structure Engineering of Highly-Scalable Earth-Abundant Multi-Synergized Electrocatalyst for Exceptional Overall Water Splitting in Neutral Medium.","description":"Efficient neutral water splitting may represent in future a sustainable solution to unconstrained energy requirements, but yet necessitates the development of innovative avenues for achieving the currently unmet required performances. Herein, a novel paradigm based on the combination of electronic structure engineering and surface morphology tuning of earth-abundant 3D-hierarchical binder-free electrocatalysts is demonstrated, via a scalable single-step thermal transformation of nickel substrates under sulfur environment. A temporal-evolution of the resulting 3D-nanostructured substrates is performed for the intentional enhancement of non-abundant highly-catalytic Ni<sup>3+</sup> and pS<sub>n</sub> <sup>2-</sup> species on the catalyst surface, concomitantly accompanied with densification ","dates":{"release":"2022-01-01T00:00:00Z","publication":"2022 Dec","modification":"2026-06-03T16:47:58.14Z","creation":"2025-04-05T21:03:13.058Z"},"accession":"S-EPMC9798964","cross_references":{"pubmed":["36366929"],"doi":["10.1002/advs.202203678"]}}