biostudies-literatureUnknown9(12)Wang CThe second-order nonlinear Hall effect observed in the time-reversal symmetric system has not only shown abundant physical content, but also exhibited potential application prospects. Recently, a third-order nonlinear Hall effect has been observed in MoTe₂ and WTe₂. However, few-layer MoTe₂ and WTe₂ are usually unstable in air and the observed third-order nonlinear Hall effect can be measured only at low temperature, which hinders further investigation as well as potential application. Thus, exploring new air-stable material systems with a sizable third-order nonlinear Hall effect at room temperature is an urgent task. Here, in type-II Weyl semimetal TaIrTe₄, we observed a pronounced third-order nonlinear Hall effect, which can exist at room temperature and remain stable for months. The third-order nonlinear Hall effect is connected to the Berry-connection polarizability tensor instead of the Berry curvature. The possible mechanism of the observation of the third-order nonlinear Hall effect in TaIrTe₄ at room temperature has been discussed. Our findings will open an avenue towards exploring room-temperature nonlinear devices in new quantum materials.National science reviewnwac020https://www.ebi.ac.uk/biostudies/studies/S-EPMC9869080biostudies-literatureRoom-temperature third-order nonlinear Hall effect in Weyl semimetal TaIrTe₄.PMC9869080Liu HYang SAWang CGao WBXiao RCCai HZhu CWang NLiu ZZhang ZLai SChen SDeng YfalseRoom-temperature third-order nonlinear Hall effect in Weyl semimetal TaIrTe₄.The second-order nonlinear Hall effect observed in the time-reversal symmetric system has not only shown abundant physical content, but also exhibited potential application prospects. Recently, a third-order nonlinear Hall effect has been observed in MoTe₂ and WTe₂. However, few-layer MoTe₂ and WTe₂ are usually unstable in air and the observed third-order nonlinear Hall effect can be measured only at low temperature, which hinders further investigation as well as potential application. Thus, exploring new air-stable material systems with a sizable third-order nonlinear Hall effect at room temperature is an urgent task. Here, in type-II Weyl semimetal TaIrTe₄, we observed a pronounced third-order nonlinear Hall effect, which can exist at room temperature and remain stable for months. The third-order nonlinear Hall effect is connected to the Berry-connection polarizability tensor instead of the Berry curvature. The possible mechanism of the observation of the third-order nonlinear Hall effect in TaIrTe₄ at room temperature has been discussed. Our findings will open an avenue towards exploring room-temperature nonlinear devices in new quantum materials.2022-01-01T00:00:00Z2022 Dec2025-04-04T12:10:38.997Z2025-02-19T03:00:31.284ZS-EPMC98690803669479910.1093/nsr/nwac020