Thickness-Dependent Interface Polarity in Infinite-Layer Nickelate Superlattices.

ABSTRACT: The interface polarity plays a vital role in the physical properties of oxide heterointerfaces because it can cause specific modifications of the electronic and atomic structure. Reconstruction due to the strong polarity of the NdNiO₂/SrTiO₃ interface in recently discovered superconducting nickelate films may play an important role, as no superconductivity has been observed in the bulk. By employing four-dimensional scanning transmission electron microscopy and electron energy-loss spectroscopy, we studied effects of oxygen distribution, polyhedral distortion, elemental intermixing, and dimensionality in NdNiO₂/SrTiO₃ superlattices grown on SrTiO₃ (001) substrates. Oxygen distribution maps show a gradual variation of the oxygen content

SUBMITTER: Yang C 

PROVIDER: S-EPMC10141440 | biostudies-literature | 2023 Apr

REPOSITORIES: biostudies-literature