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Remarkably and stable catalytic activity in reduction of 4-nitrophenol by sodium sesquicarbonate-supporting Fe2O3@Pt.

ABSTRACT: Reasonable design of bimetallic nanomaterials with support is beneficial to improve catalytic performance. This work reports a new kind of sodium sesquicarbonate-supporting Fe2O3@Pt via etching Fe3O4@Pt@SiO2, which exhibits highly efficient and stable catalytic reduction performance towards 4-NP. Sodium sesquicarbonate-supporting Fe2O3@Pt has an interconnected one-dimensional network structure that provides sufficient channels for mass transfer. At the same time, a large amount of Fe2O3@Pt is exposed on its surface, which hinders the aggregation of pt clusters and Fe2O3 nanoparticles, and facilitates the direct contact of Fe2O3@Pt reaction sites with reactant molecules, thus improving the catalytic rate of 4-NP reduction reaction. Moreover, the introduction of non-metallic Fe can not only reduce the consumption of precious metal Pt, but also improve the catalytic efficiency due to the synergistic effect. This study opens up a new avenue to develop robust catalysts for heterogeneous catalytic reactions.

SUBMITTER: Xu X 

PROVIDER: S-EPMC10155080 | biostudies-literature | 2023 May

REPOSITORIES: biostudies-literature

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Remarkably and stable catalytic activity in reduction of 4-nitrophenol by sodium sesquicarbonate-supporting Fe<sub>2</sub>O<sub>3</sub>@Pt.

Xu Xia X   Li Mingqiang M   Yang Liming L   Hu Bing B  

RSC advances 20230503 20

Reasonable design of bimetallic nanomaterials with support is beneficial to improve catalytic performance. This work reports a new kind of sodium sesquicarbonate-supporting Fe<sub>2</sub>O<sub>3</sub>@Pt <i>via</i> etching Fe<sub>3</sub>O<sub>4</sub>@Pt@SiO<sub>2</sub>, which exhibits highly efficient and stable catalytic reduction performance towards 4-NP. Sodium sesquicarbonate-supporting Fe<sub>2</sub>O<sub>3</sub>@Pt has an interconnected one-dimensional network structure that provides suffi  ...[more]

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