Ontology highlight
ABSTRACT:
SUBMITTER: Zhou C
PROVIDER: S-EPMC10275871 | biostudies-literature | 2023 Jun
REPOSITORIES: biostudies-literature
Zhou Chengxin C Gao Jian J Deng Yunlong Y Wang Ming M Li Dan D Xia Chuan C
Nature communications 20230616 1
Photocatalytic hydrogen evolution efficiency is limited due to unfavorable carrier dynamics and thermodynamic performance. Here, we propose to introduce electronegative molecules to build an electric double layer (EDL) to generate a polarization field instead of the traditional built-in electric field to improve carrier dynamics, and optimize the thermodynamics by regulating the chemical coordination of surface atoms. Based on theoretical simulation, we designed CuNi@EDL and applied it as the co ...[more]