Probing the Activity Enhancement of Carbocatalyst with the Anchoring of Atomic Metal.

ABSTRACT: Enhanced catalysis for organic transformation is essential for the synthesis of high-value compounds. Atomic metal species recently emerged as highly effective catalysts for organic reactions with high activity and metal utilization. However, developing efficient atomic catalysts is always an attractive and challenging topic in the modern chemical industry. In this work, we report the preparation and activity enhancement of nitrogen- and sulfur-codoped holey graphene (NSHG) with the anchoring of atomic metal Pd. When employed as the catalyst for nitroarenes reduction reactions, the resultant Pd/NSHG composite exhibits remarkably high catalytic activity due to the co-existence of dual-active components (i.e., catalytically active NSHG support and homogeneous dispersion of atomic metal Pd).

SUBMITTER: Zhang Z 

PROVIDER: S-EPMC10489856 | biostudies-literature | 2023 Aug

REPOSITORIES: biostudies-literature