Kapitza-resistance-like exciton dynamics in atomically flat MoSe2-WSe2 lateral heterojunction.
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ABSTRACT: Being able to control the neutral excitonic flux is a mandatory step for the development of future room-temperature two-dimensional excitonic devices. Semiconducting Monolayer Transition Metal Dichalcogenides (TMD-ML) with extremely robust and mobile excitons are highly attractive in this regard. However, generating an efficient and controlled exciton transport over long distances is a very challenging task. Here we demonstrate that an atomically sharp TMD-ML lateral heterostructure (MoSe2-WSe2) transforms the isotropic exciton diffusion into a unidirectional excitonic flow through the junction. Using tip-enhanced photoluminescence spectroscopy (TEPL) and a modified exciton transfer model, we show a discontinuity of the exciton density distribution on each side of the
SUBMITTER: Lamsaadi H
PROVIDER: S-EPMC10514293 | biostudies-literature | 2023 Sep
REPOSITORIES: biostudies-literature
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