Long-Range and High-Efficiency Plasmon-Assisted Forster Resonance Energy Transfer.

ABSTRACT: The development of a long-range and efficient Förster resonance energy transfer (FRET) process is essential for its application in key enabling optoelectronic and sensing technologies. Via controlling the delocalization of the donor's electric field and Purcell enhancements, we experimentally demonstrate long-range and high-efficiency Förster resonance energy transfer using a plasmonic nanogap formed between a silver nanoparticle and an extended silver film. Our measurements show that the FRET range can be extended to over 200 nm while keeping the FRET efficiency over 0.38, achieving an efficiency enhancement factor of ∼108 with respect to a homogeneous environment. Reducing Purcell enhancements by removing the extended silver film increases the FRET efficiency to 0.55, at the expense of t

SUBMITTER: Hamza AO 

PROVIDER: S-EPMC10641858 | biostudies-literature | 2023 Nov

REPOSITORIES: biostudies-literature