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Competing charge-density wave instabilities in the kagome metal ScV6Sn6.


ABSTRACT: Owing to its unique geometry, the kagome lattice hosts various many-body quantum states including frustrated magnetism, superconductivity, and charge-density waves (CDWs). In this work, using inelastic X-ray scattering, we discover a dynamic short-range [Formula: see text] CDW that is dominant in the kagome metal ScV6Sn6 above TCDW ≈ 91 K, competing with the [Formula: see text] CDW that orders below TCDW. The competing CDW instabilities lead to an unusual CDW formation process, with the most pronounced phonon softening and the static CDW occurring at different wavevectors. First-principles calculations indicate that the [Formula: see text] CDW is energetically favored, while a wavevector-dependent electron-phonon coupling (EPC) promotes the [Form

SUBMITTER: Cao S 

PROVIDER: S-EPMC10667248 | biostudies-literature | 2023 Nov

REPOSITORIES: biostudies-literature