Cavity-Tuned Exciton Dynamics in Transition Metal Dichalcogenides Monolayers.

ABSTRACT: A fully quantum, numerically accurate methodology is presented for the simulation of the exciton dynamics and time-resolved fluorescence of cavity-tuned two-dimensional (2D) materials at finite temperatures. This approach was specifically applied to a monolayer WSe2 system. Our methodology enabled us to identify the dynamical and spectroscopic signatures of polaronic and polaritonic effects and to elucidate their characteristic timescales across a range of exciton-cavity couplings. The approach employed can be extended to simulation of various cavity-tuned 2D materials, specifically for exploring finite temperature nonlinear spectroscopic signals.

SUBMITTER: Shen K 

PROVIDER: S-EPMC11356741 | biostudies-literature | 2024 Aug

REPOSITORIES: biostudies-literature