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Bio-based poly(benzimidazole-co-amide)-derived N, O co-doped carbons as fast-charging anodes for lithium-ion batteries.


ABSTRACT: Lithium-ion batteries (LIBs) that can be charged faster while delivering high capacity are currently in significant demand, especially for electric vehicle applications. In this context, this study introduces a less-explored subject: nitrogen and oxygen dual-doped carbons derived from bio-based copolymers, specifically poly(benzimidazole-co-amide). The synthesis involved varying proportions of benzimidazole to amide, namely, 8.5 : 1.5, 7 : 3, and 5 : 5. The copolymers were pyrolyzed under a nitrogen atmosphere to obtain co-doped carbons, wherein the copolymers acted as single sources of carbon, nitrogen, and oxygen, with the nitrogen content ranging between 12.1 and 8.0 at% and oxygen doping between 11.8 and 25.0 at%, and were named as pyrolyzed polybenzimidazole-co-amide 8.5

SUBMITTER: Patnaik KS 

PROVIDER: S-EPMC11376043 | biostudies-literature | 2024 Aug

REPOSITORIES: biostudies-literature