Dissipative Self-Assembly of Patchy Particles under Nonequilibrium Drive: A Computational Study.

ABSTRACT: Inspired by biology and implemented using nanotechnology, the self-assembly of patchy particles has emerged as a pivotal mechanism for constructing complex structures that mimic natural systems with diverse functionalities. Here, we explore the dissipative self-assembly of patchy particles under nonequilibrium conditions, with the aim of overcoming the constraints imposed by equilibrium assembly. Utilizing extensive Monte Carlo (MC) and Molecular Dynamics (MD) simulations, we provide insight into the effects of external forces that mirror natural and chemical processes on the assembly rates and the stability of the resulting assemblies comprising 8, 10, and 13 patchy particles. Implemented by a favorable bond-promoting drive in MC or a pulsed square wave potential in MD, our simulations re

SUBMITTER: Nag S 

PROVIDER: S-EPMC11500309 | biostudies-literature | 2024 Oct

REPOSITORIES: biostudies-literature