Interactions and ultrafast dynamics of exciton complexes in a monolayer semiconductor with electron gas.

ABSTRACT: We present femtosecond pump-probe measurements of neutral and charged exciton optical response in monolayer MoSe₂ to resonant photoexcitation of a given exciton state in the presence of 2D electron gas. We show that creation of charged exciton (X^-) population in a given K⁺, K^- valley requires the capture of available free carriers in the opposite valley and reduces the interaction of neutral exciton (X) with the electron Fermi sea. We also observe spectral broadening of the X transition line with the increasing X^- population caused by efficient scattering and excitation induced dephasing. From the valley-resolved analysis of the observed effects we are able to extract the spin-valley relaxation times of free carriers as a function of c

SUBMITTER: Rodek A 

PROVIDER: S-EPMC11501221 | biostudies-literature | 2024 Feb

REPOSITORIES: biostudies-literature