Probing plexciton emission from 2D materials on gold nanotrenches.

ABSTRACT: Probing strongly coupled quasiparticle excitations at their intrinsic length scales offers unique insights into their properties and facilitates the design of devices with novel functionalities. In this work, we investigate the formation and emission characteristics of plexcitons, arising from the interaction between surface plasmons in narrow gold nanotrenches and excitons in monolayer WSe₂. We study this strong plasmon-exciton coupling in both the far-field and the near-field. Specifically, we observe a Rabi splitting in the far-field reflection spectra of about 80 meV under ambient conditions, consistent with our theoretical modeling. Using a custom-designed near-field probe, we find that plexciton emission originates predominantly from the lower-frequency branch, which we ca

SUBMITTER: Zhou J 

PROVIDER: S-EPMC11541865 | biostudies-literature | 2024 Nov

REPOSITORIES: biostudies-literature