Low-Temperature Electron Spin Resonance Study of MnPS₃ Antiferromagnetic Single Crystal.

ABSTRACT: van der Waals MnPS₃ compound belonging to the class of Néel-type antiferromagnets (AFM) has recently emerged as a promising two-dimensional material for spintronic applications. In this study, we report on the electron spin resonance (ESR) study of an MnPS₃ single crystal across the Néel transition temperature (T _N = 78 K) for the magnetic field applied in the directions parallel and perpendicular to the crystallographic c axis. Furthermore, the ESR angular dependence at a temperature near T _N has been investigated. We observed multiple resonance modes with antiferromagnetic, ferromagnetic, and paramagnetic characters. In addition, we revealed the occurrence of complex spin-spin correlations and a magnetic-topological Berezin

SUBMITTER: Moro F 

PROVIDER: S-EPMC11573119 | biostudies-literature | 2024 Nov

REPOSITORIES: biostudies-literature