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Multistage Regulation Strategy via Fluorine-Rich Small Molecules for Realizing High-Performance Perovskite Solar Cells.


ABSTRACT: Perovskite solar cells (PSCs) are an ideal candidate for next-generation photovoltaic applications but face many challenges for their wider application, including uncontrolled fast crystallization, trap-assisted nonradiative recombination, and inefficient charge transport. Herein, a multistage regulation (MSR) strategy for addressing these challenges is proposed via the introduction of fluorine-rich small molecules with multiple active points (i.e., 1-[Bis(trifluoromethanesulfonyl)methyl]- 2,3,4,5,6-pentafluorobenzene (TFSP)) into the precursor solution of the perovskite film. The addition of TFSP effectively delays and regulates the crystallization and growth process of the perovskite film for larger grains and fewer defects, and it effectively improves the coverage of self-assembled mole

SUBMITTER: Chang X 

PROVIDER: S-EPMC11791946 | biostudies-literature | 2025 Feb

REPOSITORIES: biostudies-literature