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Correlated states controlled by a tunable van Hove singularity in moire WSe2 bilayers.


ABSTRACT: Twisted transition metal dichalcogenide (TMD) bilayers have enabled the discovery of superconductivity, ferromagnetism, correlated insulators, and a series of new topological phases of matter. However, the connection between these electronic phases of matter and the underlying band structure singularities has remained largely unexplored. Here, combining magnetic circular dichroism and exciton sensing measurements, we investigate the influence of a van Hove singularity (vHS) on the correlated phases in bilayer WSe2 with twist angle between 2 and 3 degrees. By tuning the vHS across the Fermi level using electric and magnetic fields, we observe Stoner ferromagnetism below moiré lattice filling one and Chern insulators at filling one. The experimental observations are supported by the continuum model band structure calculations. Our results highlight the prospect of engineering electronic phases of matter in moiré materials by tunable van Hove singularities.

SUBMITTER: Knuppel P 

PROVIDER: S-EPMC11861663 | biostudies-literature | 2025 Feb

REPOSITORIES: biostudies-literature

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Correlated states controlled by a tunable van Hove singularity in moiré WSe<sub>2</sub> bilayers.

Knüppel Patrick P   Zhu Jiacheng J   Xia Yiyu Y   Xia Zhengchao Z   Han Zhongdong Z   Zeng Yihang Y   Watanabe Kenji K   Taniguchi Takashi T   Shan Jie J   Mak Kin Fai KF  

Nature communications 20250225 1


Twisted transition metal dichalcogenide (TMD) bilayers have enabled the discovery of superconductivity, ferromagnetism, correlated insulators, and a series of new topological phases of matter. However, the connection between these electronic phases of matter and the underlying band structure singularities has remained largely unexplored. Here, combining magnetic circular dichroism and exciton sensing measurements, we investigate the influence of a van Hove singularity (vHS) on the correlated pha  ...[more]

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