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Quantum spin liquid from electron-phonon coupling.


ABSTRACT: A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "nonengineered" microscopic model (or in any material) remains challenging. Here, using numerically exact sign-problem-free quantum Monte Carlo simulations, we show that a QSL arises in a nonengineered electron-phonon model. Specifically, we investigate the ground-state phase diagram of the bond Su-Schrieffer-Heeger model on a 2D triangular lattice at (one electron per site), which we show includes a QSL phase which is fully gapped, exhibits no symmetry-breaking order, and supports deconfined fractionalized holon excitations. This suggests promising routes for finding QSLs in realistic materials and high-Tc superconductivity by lightly doping them.

SUBMITTER: Cai X 

PROVIDER: S-EPMC12377744 | biostudies-literature | 2025 Aug

REPOSITORIES: biostudies-literature

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Quantum spin liquid from electron-phonon coupling.

Cai Xun X   Han Zhaoyu Z   Li Zi-Xiang ZX   Kivelson Steven A SA   Yao Hong H  

Proceedings of the National Academy of Sciences of the United States of America 20250811 33


A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "nonengineered" microscopic model (or in any material) remains challenging. Here, using numerically exact sign-problem-free quantum Monte Carlo simulations, we show that a QSL arises in a nonengineered electron-phonon model. Specifically, we investigate the ground-state phase diagram of the bond Su-Schrieffer-He  ...[more]

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