Star-branched polymer donors enabling high-performance organic solar cells with superior flexibility and intrinsic stretchability.

ABSTRACT: Emerging wearable electronics are anticipated to leverage the flexibility and stretchability of organic solar cells (OSCs). However, achieving a balance between power conversion efficiency (PCE) and mechanical robustness remains challenging, as the molecular structural modifications required for enhanced flexibility of photovoltaic materials typically compromise charge transport and extraction. Herein, we design and synthesize three star-branched polymer donors (SPDs: S1, S2, and S3) by introducing different contents of 1,3,5-tris(bromomethyl)benzene, which boost fracture strain compared to the linear PM6 (12.70%, 15.33% and 19.16% to 10.46%), improving devices' stress resistance/fatigue endurance. More importantly, these SPDs are able to self-assemble into refined fibrous architectures to

SUBMITTER: Zhang C 

PROVIDER: S-EPMC12630945 | biostudies-literature | 2025 Nov

REPOSITORIES: biostudies-literature