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Direct Electrochemical Regeneration of Lithium-Ion Battery Cathode Material through Molecular Wiring.


ABSTRACT: Increasing use of lithium-ion batteries (LIBs) urges for efficient recycling strategies for their components. Direct recycling methods for cathode materials, based on repairing the structure of the degraded cathode particles without destroying the bulk phase, are promising energy-saving alternatives to traditional metallurgy processes that involve several steps and use large volumes of chemicals causing secondary pollution. Herein, we report a novel and scalable method for the direct electrochemical recycling of spent lithium iron phosphate (LFP) powder in a flow cell via redox mediation. In this method, pellets of spent LFP powder (S-LFP) placed in a tank are directly reduced and relithiated by a redox mediator dissolved in a Li-containing aqueous electrolyte, pumped from an electrochemic

SUBMITTER: Marin-Tajadura G 

PROVIDER: S-EPMC12767269 | biostudies-literature | 2026 Jan

REPOSITORIES: biostudies-literature