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Continuous injection synthesis of indium arsenide quantum dots emissive in the short-wavelength infrared.


ABSTRACT: With the emergence of applications based on short-wavelength infrared light, indium arsenide quantum dots are promising candidates to address existing shortcomings of other infrared-emissive nanomaterials. However, III-V quantum dots have historically struggled to match the high-quality optical properties of II-VI quantum dots. Here we present an extensive investigation of the kinetics that govern indium arsenide nanocrystal growth. Based on these insights, we design a synthesis of large indium arsenide quantum dots with narrow emission linewidths. We further synthesize indium arsenide-based core-shell-shell nanocrystals with quantum yields up to 82% and improved photo- and long-term storage stability. We then demonstrate non-invasive through-skull fluorescence imaging of the brain vascula

SUBMITTER: Franke D 

PROVIDER: S-EPMC5114595 | biostudies-literature | 2016 Nov

REPOSITORIES: biostudies-literature