Ambiguity in the causes for decadal trends in atmospheric methane and hydroxyl.

ABSTRACT: Methane is the second strongest anthropogenic greenhouse gas and its atmospheric burden has more than doubled since 1850. Methane concentrations stabilized in the early 2000s and began increasing again in 2007. Neither the stabilization nor the recent growth are well understood, as evidenced by multiple competing hypotheses in recent literature. Here we use a multispecies two-box model inversion to jointly constrain 36 y of methane sources and sinks, using ground-based measurements of methane, methyl chloroform, and the C¹³/C¹² ratio in atmospheric methane (δ¹³CH₄) from 1983 through 2015. We find that the problem, as currently formulated, is underdetermined and solutions obtained in previous work are strongly dependent on prior assumptions. Based

SUBMITTER: Turner AJ 

PROVIDER: S-EPMC5448216 | biostudies-literature | 2017 May

REPOSITORIES: biostudies-literature