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Large spontaneous exchange bias in a weak ferromagnet Pb6Ni9(TeO6)5.


ABSTRACT: We report the magnetic and dielectric behavior of Pb6Ni9(TeO6)5, a new compound comprising the honeycomb-like layers of S = 1 spins, through detailed structural, magnetic and dielectric investigation. An antiferromagnetic-type transition at 25 K (T N ) with weak-ferromagnetic behavior is revealed. Interestingly, a large value of coercive field of 1.32 T at 2 K is observed. The isothermal magnetization after zero-field-cooled condition, it exhibits the presence of large spontaneous exchange bias (SEB) with a magnitude of 0.19 T at 2 K; which is rare in single bulk materials, especially without external doping. The value of |H EB| further enhances to 0.24 T under 16 T field-cooled condition, confirming the presence of large exchange bias in the material.

SUBMITTER: Koteswararao B 

PROVIDER: S-EPMC5557810 | biostudies-literature | 2017 Aug

REPOSITORIES: biostudies-literature

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Large spontaneous exchange bias in a weak ferromagnet Pb<sub>6</sub>Ni<sub>9</sub>(TeO<sub>6</sub>)<sub>5</sub>.

Koteswararao B B   Chakrabarty Tanmoy T   Basu Tathamay T   Hazra Binoy Krishna BK   Srinivasarao P V PV   Paulose P L PL   Srinath S S  

Scientific reports 20170815 1


We report the magnetic and dielectric behavior of Pb<sub>6</sub>Ni<sub>9</sub>(TeO<sub>6</sub>)<sub>5</sub>, a new compound comprising the honeycomb-like layers of S = 1 spins, through detailed structural, magnetic and dielectric investigation. An antiferromagnetic-type transition at 25 K (T <sub>N</sub> ) with weak-ferromagnetic behavior is revealed. Interestingly, a large value of coercive field of 1.32 T at 2 K is observed. The isothermal magnetization after zero-field-cooled condition, it ex  ...[more]

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