Multidimensional photon correlation spectroscopy of cavity polaritons.

ABSTRACT: The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency-resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes-Cummings model.

SUBMITTER: Dorfman KE 

PROVIDER: S-EPMC5816200 | biostudies-literature | 2018 Feb

REPOSITORIES: biostudies-literature