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CdSe Quantum Dots/g-C3N4 Heterostructure for Efficient H2 Production under Visible Light Irradiation.


ABSTRACT: Novel photocatalysts -CdSe quantum dots (QDs)/g-C3N4- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C3N4 photocatalysts exhibited remarkably enhanced photocatalytic activity for visible-light-induced H2 evolution compared to pristine g-C3N4 and CdSe QDs and addition of 13.6 wt % CdSe QDs into the composite photocatalyst generated the highest H2 production rate. The enhanced photocatalytic performance of CdSe QDs/g-C3N4 can be attributed to the synergistic effects of excellent visible absorption and high charge separation efficiency from the heterostructure. This work could not only provide a facile method to fabricate semiconductor QDs-modified g-C3N4 photocatalysts but also contribute to the design for heterostructures.

SUBMITTER: Zhong Y 

PROVIDER: S-EPMC6643951 | biostudies-literature | 2018 Dec

REPOSITORIES: biostudies-literature

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CdSe Quantum Dots/g-C<sub>3</sub>N<sub>4</sub> Heterostructure for Efficient H<sub>2</sub> Production under Visible Light Irradiation.

Zhong Yunqian Y   Chen Weiwei W   Yu Shan S   Xie Zhanghui Z   Wei Shiqian S   Zhou Ying Y  

ACS omega 20181219 12


Novel photocatalysts -CdSe quantum dots (QDs)/g-C<sub>3</sub>N<sub>4</sub>- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C<sub>3</sub>N<sub>4</sub> photocatalysts exhibited remarkably enhanced photocatalytic activity for visible-light-induced H<sub>2</sub> evolution compared to pristine g-C<sub>3</sub>N<sub>4</sub> and CdSe QDs  ...[more]

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