MoS₂ pixel arrays for real-time photoluminescence imaging of redox molecules.

ABSTRACT: Measuring the behavior of redox-active molecules in space and time is crucial for understanding chemical and biological systems and for developing new technologies. Optical schemes are noninvasive and scalable, but usually have a slow response compared to electrical detection methods. Furthermore, many fluorescent molecules for redox detection degrade in brightness over long exposure times. Here, we show that the photoluminescence of "pixel" arrays of monolayer MoS₂ can image spatial and temporal changes in redox molecule concentration. Because of the strong dependence of MoS₂ photoluminescence on doping, changes in the local chemical potential substantially modulate the photoluminescence of MoS₂, with a sensitivity of 0.9 mV / Hz on a 5 μm × 5 μm pixel

SUBMITTER: Reynolds MF 

PROVIDER: S-EPMC6839941 | biostudies-literature | 2019 Nov

REPOSITORIES: biostudies-literature