Isotopic ratios of uranium and caesium in spherical radioactive caesium-bearing microparticles derived from the Fukushima Dai-ichi Nuclear Power Plant.

ABSTRACT: Spherical radioactive caesium (Cs)-bearing microparticles (CsMPs) were emitted during the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident in March, 2011. The emission source (timing) and formation process of these particles remain unclear. In this study, the isotopic ratios of uranium (²³⁵U and ²³⁸U) and caesium (¹³³Cs, ¹³⁴Cs, ¹³⁵Cs, and ¹³⁷Cs) isotopes in the five spherical CsMPs (ca. 2 μm in size) sampled at 50 km west of the FDNPP were determined using secondary ion mass spectrometry and laser ablation-ICPMS, respectively. Results showed that the ²³⁵U/²³⁸U ratios of CsMPs were homogeneous (1.93 ± 0.03, N = 4) and close to those estimated for the fuel cores in units 2 and 3, and that the Cs is

SUBMITTER: Kurihara Y 

PROVIDER: S-EPMC7039901 | biostudies-literature | 2020 Feb

REPOSITORIES: biostudies-literature