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Inverse ZrO₂/Cu as a highly efficient methanol synthesis catalyst from CO₂ hydrogenation.

ABSTRACT: Enhancing the intrinsic activity and space time yield of Cu based heterogeneous methanol synthesis catalysts through CO₂ hydrogenation is one of the major topics in CO₂ conversion into value-added liquid fuels and chemicals. Here we report inverse ZrO₂/Cu catalysts with a tunable Zr/Cu ratio have been prepared via an oxalate co-precipitation method, showing excellent performance for CO₂ hydrogenation to methanol. Under optimal condition, the catalyst composed by 10% of ZrO₂ supported over 90% of Cu exhibits the highest mass-specific methanol formation rate of 524 g_MeOHkg_cat^-1h^-1 at 220 °C, 3.3 times higher than the activity of traditional Cu/ZrO₂ catalysts (159 g_MeOHkg

SUBMITTER: Wu C

PROVIDER: S-EPMC7666171 | biostudies-literature | 2020 Nov

REPOSITORIES: biostudies-literature

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Inverse ZrO₂/Cu as a highly efficient methanol synthesis catalyst from CO₂ hydrogenation.

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Inverse ZrO2/Cu as a highly efficient methanol synthesis catalyst from CO2 hydrogenation.

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Inverse ZrO₂/Cu as a highly efficient methanol synthesis catalyst from CO₂ hydrogenation.