Low threshold lasing emissions from a single upconversion nanocrystal.

ABSTRACT: Cross-relaxation among neighboring emitters normally causes self-quenching and limits the brightness of luminescence. However, in nanomaterials, cross-relaxation could be well-controlled and employed for increasing the luminescence efficiency at specific wavelengths. Here we report that cross-relaxation can modulate both the brightness of single upconversion nanoparticles and the threshold to reach population inversion, and both are critical factors in producing the ultra-low threshold lasing emissions in a micro cavity laser. By homogenously coating a 5-μm cavity with a single layer of nanoparticles, we demonstrate that doping Tm³⁺ ions at 2% can facilitate the electron accumulation at the intermediate state of ³H₄ level and efficiently decrease the lasing

SUBMITTER: Shang Y 

PROVIDER: S-EPMC7708641 | biostudies-literature | 2020 Dec

REPOSITORIES: biostudies-literature