Atomically thin photoanode of InSe/graphene heterostructure.

ABSTRACT: Achieving high-efficiency photoelectrochemical water splitting requires a better understanding of ion kinetics, e.g., diffusion, adsorption and reactions, near the photoelectrode's surface. However, with macroscopic three-dimensional electrodes, it is often difficult to disentangle the contributions of surface effects to the total photocurrent from that of various factors in the bulk. Here, we report a photoanode made from a InSe crystal monolayer that is encapsulated with monolayer graphene to ensure high stability. We choose InSe among other photoresponsive two-dimensional (2D) materials because of its unique properties of high mobility and strongly suppressing electron-hole pair recombination. Using the atomically thin electrodes, we obtained a photocurrent with a density >10 mA cm

SUBMITTER: Zheng H 

PROVIDER: S-EPMC7782821 | biostudies-literature | 2021 Jan

REPOSITORIES: biostudies-literature