Probing subwavelength in-plane anisotropy with antenna-assisted infrared nano-spectroscopy.

ABSTRACT: Infrared nano-spectroscopy based on scattering-type scanning near-field optical microscopy (s-SNOM) is commonly employed to probe the vibrational fingerprints of materials at the nanometer length scale. However, due to the elongated and axisymmetric tip shank, s-SNOM is less sensitive to the in-plane sample anisotropy in general. In this article, we report an easy-to-implement method to probe the in-plane dielectric responses of materials with the assistance of a metallic disk micro-antenna. As a proof-of-concept demonstration, we investigate here the in-plane phonon responses of two prototypical samples, i.e. in (100) sapphire and x-cut lithium niobate (LiNbO₃). In particular, the sapphire in-plane vibrations between 350 cm^-1 to 800 cm^-1 that correspond to

SUBMITTER: Yao Z 

PROVIDER: S-EPMC8113487 | biostudies-literature | 2021 May

REPOSITORIES: biostudies-literature