Lignin-Based Porous Supraparticles for Carbon Capture.

ABSTRACT: Multiscale carbon supraparticles (SPs) are synthesized by soft-templating lignin nano- and microbeads bound with cellulose nanofibrils (CNFs). The interparticle connectivity and nanoscale network in the SPs are studied after oxidative thermostabilization of the lignin/CNF constructs. The carbon SPs are formed by controlled sintering during carbonization and develop high mechanical strength (58 N·mm^-3) and surface area (1152 m²·g^-1). Given their features, the carbon SPs offer hierarchical access to adsorption sites that are well suited for CO₂ capture (77 mg CO₂·g^-1), while presenting a relatively low pressure drop (∼33 kPa·m^-1 calculated for a packed fixed-bed column). The introduced lignin-derived SPs address the

SUBMITTER: Zhao B 

PROVIDER: S-EPMC8155330 | biostudies-literature | 2021 Apr

REPOSITORIES: biostudies-literature