Quadrupolar charge dynamics in the nonmagnetic FeSe_1-x S _x superconductors.

ABSTRACT: We use polarization-resolved electronic Raman spectroscopy to study quadrupolar charge dynamics in a nonmagnetic [Formula: see text] superconductor. We observe two types of long-wavelength [Formula: see text] symmetry excitations: 1) a low-energy quasi-elastic scattering peak (QEP) and 2) a broad electronic continuum with a maximum at 55 meV. Below the tetragonal-to-orthorhombic structural transition at [Formula: see text], a pseudogap suppression with temperature dependence reminiscent of the nematic order parameter develops in the [Formula: see text] symmetry spectra of the electronic excitation continuum. The QEP exhibits critical enhancement upon cooling toward [Formula: see text] The intensity of the QEP grows with increasing sulfur concentration x and maximizes near critical concentr

SUBMITTER: Zhang W 

PROVIDER: S-EPMC8157944 | biostudies-literature | 2021 May

REPOSITORIES: biostudies-literature