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Solar-driven tandem photoredox nickel-catalysed cross-coupling using modified carbon nitride.


ABSTRACT: Nickel-catalysed aryl amination and etherification are driven with sunlight using a surface-modified carbon nitride to extend the absorption of the photocatalyst into a wide range of the visible region. In contrast to traditional homogeneous photochemical methodologies, the lower cost and higher recyclability of the metal-free photocatalyst, along with the use of readily available sunlight, provides an efficient and sustainable approach to promote nickel-catalysed cross-couplings.

SUBMITTER: Qin Y 

PROVIDER: S-EPMC8159281 | biostudies-literature | 2020 Jun

REPOSITORIES: biostudies-literature

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Solar-driven tandem photoredox nickel-catalysed cross-coupling using modified carbon nitride.

Qin Yangzhong Y   Martindale Benjamin C M BCM   Sun Rui R   Rieth Adam J AJ   Nocera Daniel G DG  

Chemical science 20200625 28


Nickel-catalysed aryl amination and etherification are driven with sunlight using a surface-modified carbon nitride to extend the absorption of the photocatalyst into a wide range of the visible region. In contrast to traditional homogeneous photochemical methodologies, the lower cost and higher recyclability of the metal-free photocatalyst, along with the use of readily available sunlight, provides an efficient and sustainable approach to promote nickel-catalysed cross-couplings. ...[more]

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