Efficient sequential harvesting of solar light by heterogeneous hollow shells with hierarchical pores.

ABSTRACT: In nature, sequential harvesting of light widely exists in the old life entity, i.e. cyanobacteria, to maximize the light absorption and enhance the photosynthesis efficiency. Inspired by nature, we propose a brand new concept of temporally-spatially sequential harvesting of light in one single particle, which has purpose-designed heterogeneous hollow multi-shelled structures (HoMSs) with porous shells composed of nanoparticle subunits. Structurally, HoMSs consist of different band-gap materials outside-in, thus realizing the efficient harvesting of light with different wavelengths. Moreover, introducing oxygen vacancies into each nanoparticle subunit can also enhance the light absorption. With the benefit of sequential harvesting of light in HoMSs, the quantum efficiency at wavelength of

SUBMITTER: Wei Y 

PROVIDER: S-EPMC8290956 | biostudies-literature | 2020 Nov

REPOSITORIES: biostudies-literature