Large ultrafast-modulated Voigt effect in noncollinear antiferromagnet Mn₃Sn.

ABSTRACT: The time-resolved magneto-optical (MO) Voigt effect can be utilized to study the Néel order dynamics in antiferromagnetic (AFM) materials, but it has been limited for collinear AFM spin configuration. Here, we have demonstrated that in Mn₃Sn with an inverse triangular spin structure, the quench of AFM order by ultrafast laser pulses can result in a large Voigt effect modulation. The modulated Voigt angle is significantly larger than the polarization rotation due to the crystal-structure related linear dichroism effect and the modulated MO Kerr angle arising from the ferroic ordering of cluster magnetic octupole. The AFM order quench time shows negligible change with increasing temperature approaching the Néel temperature (T_N), in markedly contrast with the pronounced

SUBMITTER: Zhao HC 

PROVIDER: S-EPMC8421456 | biostudies-literature | 2021 Sep

REPOSITORIES: biostudies-literature