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Supramolecular photocatalysts fixed on the inside of the polypyrrole layer in dye sensitized molecular photocathodes: application to photocatalytic CO₂ reduction coupled with water oxidation.

ABSTRACT: The development of systems for photocatalytic CO₂ reduction with water as a reductant and solar light as an energy source is one of the most important milestones on the way to artificial photosynthesis. Although such reduction can be performed using dye-sensitized molecular photocathodes comprising metal complexes as redox photosensitizers and catalyst units fixed on a p-type semiconductor electrode, the performance of the corresponding photoelectrochemical cells remains low, e.g., their highest incident photon-to-current conversion efficiency (IPCE) equals 1.2%. Herein, we report a novel dye-sensitized molecular photocathode for photocatalytic CO₂ reduction in water featuring a polypyrrole layer, [Ru(diimine)₃]²⁺ as a redox photosensitize

SUBMITTER: Kuttassery F

PROVIDER: S-EPMC8513877 | biostudies-literature | 2021 Oct

REPOSITORIES: biostudies-literature

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Supramolecular photocatalysts fixed on the inside of the polypyrrole layer in dye sensitized molecular photocathodes: application to photocatalytic CO₂ reduction coupled with water oxidation.

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Supramolecular photocatalysts fixed on the inside of the polypyrrole layer in dye sensitized molecular photocathodes: application to photocatalytic CO2 reduction coupled with water oxidation.

OmicsDI is part of the ELIXIR infrastructure

Tweets

Supramolecular photocatalysts fixed on the inside of the polypyrrole layer in dye sensitized molecular photocathodes: application to photocatalytic CO₂ reduction coupled with water oxidation.