Exciton-polaron Rydberg states in monolayer MoSe₂ and WSe₂.

ABSTRACT: Exciton polaron is a hypothetical many-body quasiparticle that involves an exciton dressed with a polarized electron-hole cloud in the Fermi sea. It has been evoked to explain the excitonic spectra of charged monolayer transition metal dichalcogenides, but the studies were limited to the ground state. Here we measure the reflection and photoluminescence of monolayer MoSe₂ and WSe₂ gating devices encapsulated by boron nitride. We observe gate-tunable exciton polarons associated with the 1 s-3 s exciton Rydberg states. The ground and excited exciton polarons exhibit comparable energy redshift (15~30 meV) from their respective bare excitons. The robust excited states contradict the trion picture because the trions are expected to dissociate in the excited states. When th

SUBMITTER: Liu E 

PROVIDER: S-EPMC8531338 | biostudies-literature | 2021 Oct

REPOSITORIES: biostudies-literature