A Silicon Monoxide Lithium-Ion Battery Anode with Ultrahigh Areal Capacity.

ABSTRACT: Silicon monoxide (SiO) is an attractive anode material for next-generation lithium-ion batteries for its ultra-high theoretical capacity of 2680 mAh g^-1. The studies to date have been limited to electrodes with a relatively low mass loading (< 3.5 mg cm^-2), which has seriously restricted the areal capacity and its potential in practical devices. Maximizing areal capacity with such high-capacity materials is critical for capitalizing their potential in practical technologies. Herein, we report a monolithic three-dimensional (3D) large-sheet holey graphene framework/SiO (LHGF/SiO) composite for high-mass-loading electrode. By specifically using large-sheet holey graphene building blocks, we construct LHGF with super-elasticity and exceptional mechanical robustness, whic

SUBMITTER: Zhong J 

PROVIDER: S-EPMC8789978 | biostudies-literature | 2022 Jan

REPOSITORIES: biostudies-literature