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Strain-mediated ferromagnetism and low-field magnetic reversal in Co doped monolayer [Formula: see text].


ABSTRACT: Strain-mediated magnetism in 2D materials and dilute magnetic semiconductors hold multi-functional applications for future nano-electronics. Herein, First principles calculations are employed to study the influence of biaxial strain on the magnetic properties of Co-doped monolayer [Formula: see text]. The non-magnetic [Formula: see text] shows ferromagnetic signature upon Co doping due to spin polarization, which is further improved at low compressive (-2 %) and tensile (+2 %) strains. From the PDOS and spin density analysis, the opposite magnetic ordering is found to be favourable under the application of compressive and tensile strains. The double exchange interaction and p-d hybridization mechanisms make Co-doped [Formula: see text] a potential host for magnetism. More importantly, the competition between exchange and crystal field splittings, i.e. ([Formula: see text]), of the Co-atom play pivotal roles in deciding the values of the magnetic moments under applied strain. Micromagnetic simulation reveals, the ferromagnetic behavior calculated from DFT exhibits low-field magnetic reversal (190 Oe). Moreover, the spins of Co-doped [Formula: see text] are slightly tilted from the easy axis orientations showing slanted ferromagnetic hysteresis loop. The ferromagnetic nature of Co-doped [Formula: see text] suppresses beyond [Formula: see text] strain, which is reflected in terms of decrease in the coercivity in the micromagnetic simulation. The understanding of low-field magnetic reversal and spin orientations in Co-doped [Formula: see text] may pave the way for next-generation spintronics and straintronics applications.

SUBMITTER: Jena AK 

PROVIDER: S-EPMC8850603 | biostudies-literature | 2022 Feb

REPOSITORIES: biostudies-literature

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Strain-mediated ferromagnetism and low-field magnetic reversal in Co doped monolayer [Formula: see text].

Jena Anjan Kumar AK   Mallik Sameer Kumar SK   Sahu Mousam Charan MC   Sahoo Sandhyarani S   Sahoo Ajit Kumar AK   Sharma Neha Kapila NK   Mohanty J J   Gupta Sanjeev K SK   Ahuja Rajeev R   Sahoo Satyaprakash S  

Scientific reports 20220216 1


Strain-mediated magnetism in 2D materials and dilute magnetic semiconductors hold multi-functional applications for future nano-electronics. Herein, First principles calculations are employed to study the influence of biaxial strain on the magnetic properties of Co-doped monolayer [Formula: see text]. The non-magnetic [Formula: see text] shows ferromagnetic signature upon Co doping due to spin polarization, which is further improved at low compressive (-2 %) and tensile (+2 %) strains. From the  ...[more]

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