Self-Assembly Dynamics of Reconfigurable Colloidal Molecules.
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ABSTRACT: Colloidal molecules are designed to mimic their molecular analogues through their anisotropic shape and interactions. However, current experimental realizations are missing the structural flexibility present in real molecules thereby restricting their use as model systems. We overcome this limitation by assembling reconfigurable colloidal molecules from silica particles functionalized with mobile DNA linkers in high yields. We achieve this by steering the self-assembly pathway toward the formation of finite-sized clusters by employing high number ratios of particles functionalized with complementary DNA strands. The size ratio of the two species of particles provides control over the overall cluster size, i.e., the number of bound particles N, as well as the degree of reconfi
SUBMITTER: Chakraborty I
PROVIDER: S-EPMC8867909 | biostudies-literature | 2022 Feb
REPOSITORIES: biostudies-literature
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