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Fully printed and multifunctional graphene-based wearable e-textiles for personalized healthcare applications.

ABSTRACT: Wearable e-textiles have gained huge tractions due to their potential for non-invasive health monitoring. However, manufacturing of multifunctional wearable e-textiles remains challenging, due to poor performance, comfortability, scalability, and cost. Here, we report a fully printed, highly conductive, flexible, and machine-washable e-textiles platform that stores energy and monitor physiological conditions including bio-signals. The approach includes highly scalable printing of graphene-based inks on a rough and flexible textile substrate, followed by a fine encapsulation to produce highly conductive machine-washable e-textiles platform. The produced e-textiles are extremely flexible, conformal, and can detect activities of various body parts. The printed in-plane supercapacitor provides an aerial capacitance of ∼3.2 mFcm^-2 (stability ∼10,000 cycles). We demonstrate such e-textiles to record brain activity (an electroencephalogram, EEG) and find comparable to conventional rigid electrodes. This could potentially lead to a multifunctional garment of graphene-based e-textiles that can act as flexible and wearable sensors powered by the energy stored in graphene-based textile supercapacitors.

SUBMITTER: Islam MR

PROVIDER: S-EPMC8914337 | biostudies-literature | 2022 Mar

REPOSITORIES: biostudies-literature

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Fully printed and multifunctional graphene-based wearable e-textiles for personalized healthcare applications.

Islam Md Rashedul MR Afroj Shaila S Beach Christopher C Islam Mohammad Hamidul MH Parraman Carinna C Abdelkader Amr A Casson Alexander J AJ Novoselov Kostya S KS Karim Nazmul N

iScience 20220218 3

Wearable e-textiles have gained huge tractions due to their potential for non-invasive health monitoring. However, manufacturing of multifunctional wearable e-textiles remains challenging, due to poor performance, comfortability, scalability, and cost. Here, we report a fully printed, highly conductive, flexible, and machine-washable e-textiles platform that stores energy and monitor physiological conditions including bio-signals. The approach includes highly scalable printing of graphene-based ...[more]

PMID: 35281734

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Project description:The demand for highly flexible and self-powered wearable textile devices has increased in recent years. Graphene coated textile-based wearable devices have been used for energy harvesting and storage due to their outstanding mechanical, electrical and electronic properties. However, the use of metal based nanocomposites is limited in textiles, due to their poor bending, fixation, and binding on textiles. We present here reduced graphene oxide (rGO) as an n-type and conductive polymer poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) as a p-type material for a wearable thermoelectric nanogenerator (TEG) using a (pad-dry-cure) technique. We developed a reduced graphene oxide (rGO) coated textile-based wearable TEG for energy harvesting from low-grade human body heat. The conductive polymer (PEDOT:PSS) and (rGO) nanocomposite were coated using a layer by layer approach. The resultant fabric showed higher weight pickup of 60-80%. The developed textile based TEG device showed an enhanced Seebeck coefficient of (25-150 μV K-1), and a power factor of (2.5-60 μW m-1 K-1). The developed TE device showed a higher potential to convert the low-grade body heat into electrical energy, between the human body temperature of (36.5 °C) and an external environment of (20.0 ± 5 °C) with a temperature difference of (2.5-16.5 °C). The wearable textile-based TEG is capable of producing an open circuit output voltage of 12.5-119.5 mV at an ambient fixed temperature of (20 °C). The rGO coated textile fabric also showed reduced electrical sheet resistance by increasing the number of dyeing cycles (10) and increased with the number of (20) washing cycles. The developed reduced graphene oxide (rGO) coated electrodes showed a sheet resistance of 185-45 kΩ and (15 kΩ) for PEDOT:PSS-rGO nanocomposites respectively. Furthermore, the mechanical performance of the as coated textile fabric was enhanced from (20-80 mPa) with increasing number of padding cycles. The thermoelectric performance was significantly improved, without influencing the breath-ability and comfort properties of the resultant fabric. This study presents a promising approach for the fabrication of PEDOT:PSS/rGO nano-hybrids for textile-based wearable thermoelectric generators (TEGs) for energy harvesting from low-grade body heat.

Dataset Information

Fully printed and multifunctional graphene-based wearable e-textiles for personalized healthcare applications.

Publications

Fully printed and multifunctional graphene-based wearable e-textiles for personalized healthcare applications.

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