Unusually large exciton binding energy in multilayered 2H-MoTe₂.

ABSTRACT: Although large exciton binding energies of typically 0.6-1.0 eV are observed for monolayer transition metal dichalcogenides (TMDs) owing to strong Coulomb interaction, multilayered TMDs yield relatively low exciton binding energies owing to increased dielectric screening. Recently, the ideal carrier-multiplication threshold energy of twice the bandgap has been realized in multilayered semiconducting 2H-MoTe₂ with a conversion efficiency of 99%, which suggests strong Coulomb interaction. However, the origin of strong Coulomb interaction in multilayered 2H-MoTe₂, including the exciton binding energy, has not been elucidated to date. In this study, unusually large exciton binding energy is observed through optical spectroscopy conducted on CVD-grown 2H-MoTe₂.

SUBMITTER: Jung E 

PROVIDER: S-EPMC8927107 | biostudies-literature | 2022 Mar

REPOSITORIES: biostudies-literature