Room-Temperature Observation of Near-Intrinsic Exciton Linewidth in Monolayer WS₂.

ABSTRACT: The homogeneous exciton linewidth, which captures the coherent quantum dynamics of an excitonic state, is a vital parameter in exploring light-matter interactions in 2D transition metal dichalcogenides (TMDs). An efficient control of the exciton linewidth is of great significance, and in particular of its intrinsic linewidth, which determines the minimum timescale for the coherent manipulation of excitons. However, such a control is rarely achieved in TMDs at room temperature (RT). While the intrinsic A exciton linewidth is down to 7 meV in monolayer WS₂ , the reported RT linewidth is typically a few tens of meV due to inevitable homogeneous and inhomogeneous broadening effects. Here, it is shown that a 7.18 meV near-intrinsic linewidth can be observed at RT when monolayer WS

SUBMITTER: Fang J 

PROVIDER: S-EPMC9012685 | biostudies-literature | 2022 Apr

REPOSITORIES: biostudies-literature