Quadrupolar magnetic excitations in an isotropic spin-1 antiferromagnet.

ABSTRACT: The microscopic origins of emergent behaviours in condensed matter systems are encoded in their excitations. In ordinary magnetic materials, single spin-flips give rise to collective dipolar magnetic excitations called magnons. Likewise, multiple spin-flips can give rise to multipolar magnetic excitations in magnetic materials with spin S ≥ 1. Unfortunately, since most experimental probes are governed by dipolar selection rules, collective multipolar excitations have generally remained elusive. For instance, only dipolar magnetic excitations have been observed in isotropic S = 1 Haldane spin systems. Here, we unveil a hidden quadrupolar constituent of the spin dynamics in antiferromagnetic S = 1 Haldane chain material Y₂BaNiO₅ using Ni L₃-edge resonant inel

SUBMITTER: Nag A 

PROVIDER: S-EPMC9051120 | biostudies-literature | 2022 Apr

REPOSITORIES: biostudies-literature