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In situ temperature measurements in sooting methane/air flames using synchrotron x-ray fluorescence of seeded krypton atoms.


ABSTRACT: Synchrotron x-ray fluorescence has been used to measure temperatures in optically dense gases where traditional methods would fail. These data provide a benchmark for stringent tests of computational fluid dynamics models for complex systems where physical and chemical processes are intimately linked. The experiments measured krypton number densities in a sooting, atmospheric pressure, nonpremixed coflow flame that is widely used in combustion research. The experiments not only form targets for the models, but the simulations also identify potential sources of uncertainties in the measurements, allowing for future improvements.

SUBMITTER: Montgomery MJ 

PROVIDER: S-EPMC9054011 | biostudies-literature | 2022 Apr

REPOSITORIES: biostudies-literature

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In situ temperature measurements in sooting methane/air flames using synchrotron x-ray fluorescence of seeded krypton atoms.

Montgomery Matthew J MJ   Kwon Hyunguk H   Kastengren Alan L AL   Pfefferle Lisa D LD   Sikes Travis T   Tranter Robert S RS   Xuan Yuan Y   McEnally Charles S CS  

Science advances 20220429 17


Synchrotron x-ray fluorescence has been used to measure temperatures in optically dense gases where traditional methods would fail. These data provide a benchmark for stringent tests of computational fluid dynamics models for complex systems where physical and chemical processes are intimately linked. The experiments measured krypton number densities in a sooting, atmospheric pressure, nonpremixed coflow flame that is widely used in combustion research. The experiments not only form targets for  ...[more]

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