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Effect of thiophene S on the enhanced ORR electrocatalytic performance of sulfur-doped graphene quantum dot/reduced graphene oxide nanocomposites.


ABSTRACT: In this study, a novel and simple hydrothermal method was developed to synthesize sulfur-doped graphene quantum dots (S-GQDs) with a diameter of 1-6 nm and S-GQD/reduced graphene oxide hybrids. The results indicated that an increase in the sulfur content led to superior ORR electrocatalytic activity. Moreover, it is found that thiophene S plays a significant role in the electrocatalytic activity. In addition, the average electron transfer number depends on the content of thiophene S. It is believed that the proposed synthesis strategy is a general and effective method for designing high-performance metal-free electrocatalytic materials.

SUBMITTER: Li F 

PROVIDER: S-EPMC9080651 | biostudies-literature | 2018 May

REPOSITORIES: biostudies-literature

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Effect of thiophene S on the enhanced ORR electrocatalytic performance of sulfur-doped graphene quantum dot/reduced graphene oxide nanocomposites.

Li Fei F   Sun Lang L   Luo Yi Y   Li Ming M   Xu Yongjie Y   Hu Guanghui G   Li Xinyu X   Wang Liang L  

RSC advances 20180529 35


In this study, a novel and simple hydrothermal method was developed to synthesize sulfur-doped graphene quantum dots (S-GQDs) with a diameter of 1-6 nm and S-GQD/reduced graphene oxide hybrids. The results indicated that an increase in the sulfur content led to superior ORR electrocatalytic activity. Moreover, it is found that thiophene S plays a significant role in the electrocatalytic activity. In addition, the average electron transfer number depends on the content of thiophene S. It is belie  ...[more]

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