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Coherent response of the electronic system driven by non-interfering laser pulses.

ABSTRACT: The strength of light-matter interaction in condensed matter is fundamentally linked to the orientation and oscillation strength of the materials' optical transition dipoles. Structurally anisotropic materials, e.g., elongated molecules, exhibit optical transition dipoles with fixed orientations that govern the angular-dependent light-matter interaction. Contrary, free electron-like metals should exhibit isotropic light-matter interaction with the light fields dictating the orientation of the optical transition dipoles. Here, we demonstrate that an anisotropic direction of the optical transition dipoles even exists in highly free electron-like noble metal surfaces. Our time- and phase-resolved photoemission experiment reveals coherent interference effects on the (110)-oriented silver surface after optical excitation with two non-interfering cross-polarized pulses. We explain this coherent material response within the density matrix formalism by an intrinsic coupling of the non-interfering light fields mediated by optical transition dipoles with fixed orientations in silver.

SUBMITTER: Eul T

PROVIDER: S-EPMC9184506 | biostudies-literature | 2022 Jun

REPOSITORIES: biostudies-literature

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Coherent response of the electronic system driven by non-interfering laser pulses.

Eul Tobias T Prinz Eva E Hartelt Michael M Frisch Benjamin B Aeschlimann Martin M Stadtmüller Benjamin B

Nature communications 20220609 1

The strength of light-matter interaction in condensed matter is fundamentally linked to the orientation and oscillation strength of the materials' optical transition dipoles. Structurally anisotropic materials, e.g., elongated molecules, exhibit optical transition dipoles with fixed orientations that govern the angular-dependent light-matter interaction. Contrary, free electron-like metals should exhibit isotropic light-matter interaction with the light fields dictating the orientation of the op ...[more]

PMID: 35680865

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Project description:We present a particle-in-cell (PIC) analysis of terahertz (THz) radiation by ultrafast plasma currents driven by relativistic-intensity laser pulses. We show that, while the I0 [Formula: see text] product of the laser intensity I0 and the laser wavelength λ0 plays the key role in the energy scaling of strong-field laser-plasma THz generation, the THz output energy, WTHz, does not follow the I0 [Formula: see text] scaling. Its behavior as a function of I0 and λ0 is instead much more complex. Our two- and three-dimensional PIC analysis shows that, for moderate, subrelativistic and weakly relativistic fields, WTHz(I0 [Formula: see text]) can be approximated as (I0λ02)α, with a suitable exponent α, as a clear signature of vacuum electron acceleration as a predominant physical mechanism whereby the energy of the laser driver is transferred to THz radiation. For strongly relativistic laser fields, on the other hand, WTHz(I0 [Formula: see text]) closely follows the scaling dictated by the relativistic electron laser ponderomotive potential [Formula: see text], converging to WTHz ∝ [Formula: see text] for very high I0, thus indicating the decisive role of relativistic ponderomotive charge acceleration as a mechanism behind laser-to-THz energy conversion. Analysis of the electron distribution function shows that the temperature Te of hot laser-driven electrons bouncing back and forth between the plasma boundaries displays the same behavior as a function of I0 and λ0, altering its scaling from (I0λ02)α to that of [Formula: see text], converging to WTHz ∝ [Formula: see text] for very high I0. These findings provide a clear physical picture of THz generation in relativistic and subrelativistic laser plasmas, suggesting the THz yield WTHz resolved as a function of I0 and λ0 as a meaningful measurable that can serve as a probe for the temperature Te of hot electrons in a vast class of laser-plasma interactions. Specifically, the α exponent of the best (I0λ02)α fit of the THz yield suggests a meaningful probe that can help identify the dominant physical mechanisms whereby the energy of the laser field is converted to the energy of plasma electrons.

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Coherent response of the electronic system driven by non-interfering laser pulses.

Publications

Coherent response of the electronic system driven by non-interfering laser pulses.

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